Circularly Polarized High-Harmonics – From Symmetries to Applications
Generation of high harmonics of light fields had led to numerous scientific and technological advancements since its discovery 30 years ago, including attosecond spectroscopy of atoms, molecules and condensed matter and tabletop high-resolution imaging of nanostructures. However, the polarization state of high harmonics was essentially limited to linear, which prevented experimental access to the role of photon-spin in harmonic generation, and hindered the use of high harmonic radiation for chiro-optical investigation with magnetic and other chiral matter.
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